CONCERT

Contrail and Cirrus Experiment

Homepage for the CONCERT Falcon campaigns in 2008 and 2011
 

Instruments on the Falcon

Click on the images below to enlarge.

AIMS Atmospheric chemical Ionization Mass Spectrometer (DLR)

The chemical ionization mass spectrometry is a highly sensitive instrument for the detection of trace gases such as HNO3, HONO, SO2, HCl and ClONO2 in the lower ppt range.
-Accuracy: ~ ± 20 % for in-flight calibrated compounds (SO2, HNO3, and Bry)
-Precision: ~ ± 5-10 %

Detection limit: few to some ten ppt

-Time resolution: 0.2 - 1s

     


NOy instrument (DLR)

NOy is the sum of reactive nitrogen species: NOy = å  NO + NO2 + HNO3 + HNO2 + N2O5+ PAN + particle nitrate + ...
Total (gasphase plus enhanced particulate) NOy is measured with a forward facing inlet, gasphase NOy with a rear facing inlet.
In brief, the detection principle of the NOy instrument is based on the evaporation of particles in the forward facing inlet, the reduction of gaseous NOy to NO with CO in a heated gold converter and the detection of the chemiluminescence reaction of NO with ozone in the near infra red. The instrumental error for NOy is +/-12%.
Temporal resolution: 1 sec
Altitude range: 0-12 km
Detection limit: 5 ppt for NOy
Sensitivity: 10 counts/ppt for NOy


Ozone detector (DLR)

The detection principle of the ozone instrument is based on UV absorption. The sample air is drawn in parallel through two reactors. O3 is removed from the sample air in one of the reactors. The sample air within the two reactors is exposed to UV radiation and the UV signal difference between both reactors is detected as a measure of the ozone concentration. 
 

    


Waran / Water vapor TDL (DLR)

WVSS-II: Tunable Diode Laser at l = 1,3  µm
range: 20-40000 ppmv
accuracy: 50 ppmv or 5%
data link to weather stations (AMDAR)
 

    


Cloud Imaging Probe (CIP, University Mainz)

This optical spectrometer measures the size and shape of particles passing through its collimated laser beam, from 25µm to 1600 µm with a resolution of 25µm. It is capable of concentrations up to 100cm-3 and airspeeds up to 200 ms-1. It uses a fast 64-element photodiode array to generate 2-dimensional images of the particles. Included in this instrument package are temperature, pressure and relative humidity sensors.

 


Forward Scattering Spectrometer Probe: FSSP-300 (DLR/University Mainz)

The FSSPs measure the forward scattering of single particles within a scattering angle of 3-15°. Using Mie-calculations, the size of a particle is related to the measured scattering cross section, which implicitly assumes spherical particles. The settings of the instruments allow determination of ice crystal size distributions in 40 size bins between 2 and 47 µm diameter (FSSP-100) and between 0.3 and  40µm (FSSP-300). Due to ambiguities in the Mie scattering curve the size distributions will be summarised in about 10 size bins.


Polar Nephelometer (PN, University Clermont-Ferrand)

The airborne Polar Nephelometer is designed to measure the optical and microphysical parameters of clouds containing either water droplets or ice crystals or a  mixture of these particles over a size range from a few micrometers to about 800 microns diameter. The airborne version of the probe is compatible with PMS canister. The probe measures the scattering phase function of an ensemble of cloud particles which intersect a collimated laser beam near the focal point of a paraboloidal mirror. The light scattered from polar angles from ±3.49 to ±169° is reflected onto a circular array of 54 photodiodes. The signal processing electronics and computer storage can provide one measurement of the scattering phase function every 10 msec. The optical properties (extinction coefficient, asymmetry factor, backscattering coefficient, ...) are derived from the measured scattering phase functions. The particle size spectra and subsequent derived quantities such bulk parameters and size parameters are retrieved using an inversion technique. The particle phase discrimination (water droplet / ice particles) can be derived from the shape of the scattering phase function.

 


HNO3/HCl mass spectrometer (DLR/MPI-K) 2008

The CIMS (Chemical Ionization Mass Spectrometry) method equipped with an Ion Trap Mass Spectrometer (ITMS) (by Finnigan LCQ, Finnigan Company USA) is a highly sensitive instrument for atmospheric measurements of the reservoir gases HNO3 and HCl in the lower ppt range. The IT-CIMS instrument has been modified and mounted on the Falcon by MPI-K and DLR using a selective ion-molecule reaction for online detection of atmospheric trace gases at low concentrations. A standard is used for in-flight-calibration, thereby reducing uncertainties arising from wall losses and ion-hydration. HCl transported down from the stratosphere into the upper troposphere can be used as a tracer for stratospheric air masses. Gaseous HNO3 in the UT/LS is simultaneously detected.

The inlet system, using a passive flow tube combined with a pressure stabilized ionisation region, has been modified and improved to account for a faster and more sensitive detection of these acids.

Temporal resolution: 2 sec
Altitude range: 6-12 km
Detection limit: 50 ppt for HCl; 80 ppt for HNO3
Sensitivity: 4.5 counts/ppt for HCl, 10 counts/ppt for HNO3


Time-of-Flight Aerosol Mass Spectrometer C-ToF-AMS (MPI-C) 2008

Specifications:

- pressure controlled inlet
- particle focusing by aerodynamic lens
- flash evaporation of non-refractory particles (600°C)
- electron impact ionization (70 eV)
- ToF MS for ion analysisSize range:ca. 40 – 1000 nm


Measured quantities:

Mass concentrations and size distributions of organics (HOA, OOA), SO4, NO3, and NH4

Time resolution:

up to 1 sec. (mass concentration mode only),
up to 10 sec. (size distributions and mass concentrations)

Detection limits (aircraft conditions):

Species               30 sec            5 min
SO4:                 0.10 µg/m3     0.03 µg/m3  
NO3:                 0.15 µg/m3     0.05 µg/m3
NH4:                 0.24 µg/m3     0.08 µg/m3
Org:                  3.0 µg/m3       0.95 µg/m3

Detection limits (standard vacuum conditions):

Species               30 sec            5 min
SO4                  0.017 µg/m3    0.006 µg/m3
NO3                  0.015 µg/m3    0.005 µg/m3
NH4                  0.18 µg/m3      0.056 µg/m3
Org                   0.83 µg/m3      0.26 µg/m3


CLOUD PARTICLE IMAGER (CPI, University Clermont-Ferrand) 2008

The CPI records very high resolution (2.3 mm) digital images of cloud particles as they pass through the sample tube of the instrument. It casts an image of the particle on a solid-state CCD camera by freezing the motion of the particle using a 25 ns pulsed, high-power laser diode. Upstream lasers precisely define the depth-of-field (DOF) so that at least one particle in the image is almost always in the focus. This eliminates out-of-focus sizing errors that have plagued the conventional 2D imaging probes. The method of data processing leads to derive the particle size distribution and calculates the usual microphysical parameters: ice particle concentration, extinction coefficient, mean particle size, radar reflectivity and ice water content. The classification of the shape of the ice particles can also be derived.

 


SMART Albedometer (University Mainz) 2008

Measured quantities

spectral upwelling radiances (W/(m² nm sr))
spectral upwelling irradiances (W/(m² nm))


Spectral upwelling radiances and irradiances are measured with the Spectral Modular Airborne Radiation measurement sysTem (SMART)-Albedometer
developed at the Leibniz Institute for Tropospheric Research (IfT), Leipzig, Germany. By connecting specific optical inlets to a set of up to six spectrometers, this instrument allows the measurement of different radiometric quantities (irradiance, radiance, actinic radiation) on airborne platforms.
During the CONCERT experiment, an optical inlet with a viewing angle of 1.5° designed to measure radiances as well as an irradiance optical inlet (half-dome shape) are each connected to two plain-grated spectrometers, respectively. The optical inlets are placed in the back part of the fuselage of the aircraft (see foto).
The spectrometers operate in the wavelength ranges 350--1050 nm and 900--2200 nm with spectral resolutions (Full Width at Half Maximum, FWHM) of 2--3 nm and 9--16 nm, respectively. The temporal resolution of the measurements is in the order of 0.5--3s, corresponding to a spatial resolution of 100--600m at an aircraft velocity of 200m/s.


FISH Fast In situ Stratospheric Hygrometer (Research Center Jülich) 2008

The Fish instrument has been developed at Forschungszentrum Jülich (Germany) to measure H2O in the upper troposphere and lower stratosphere. It mainly consists of
- a Lyman-alpha radiation source
- a mirror drive
- a fluorescence cell
- two VUV radiation detectors (NO-cells)
- and a photomultiplier tube (PMT) as optical part.

The instrument is closed and the measuring system is based on the Lyman-alpha photofragment fluorescence technique:
Radiation with a wavelength of 121,6 lambda is emitted by a lamp which is filled with a H2/Ar-mixture. To avoid contamination of the fluorescence cell due to the lamp-gas a MgF2-window is placed in the outlet of the lamp to make it tight. The Lyman-alpha radiation gets to a mirror-drive, where three different mirror-positions enable to determine the background, the intensity of the Lyman-alpha radiation and the dark counts with the VUV detectors and the PMT. In the fluorescence cell the H2O-molecules of the moist air are now photodissociated by the high-energetic radiation, thus electronically excited OH is produced.

H20 + hv ----> OH* + H ; if lambda < 137nm

Since OH relaxes to the ground state, fluorescence radiation is emitted.

OH* ----> OH + hv ; if 280 < lambda < 330nm

Because fluorescence-photons and water-mixing ratio are proportional, measurements of fluorescence are used to determine humidity of the air.
With a measurement frequency of 1 Hz, the noise equivalent mixing ratio at 3 ppmv is 0.2-0.15 ppmv, and the detection limit is 0.18-0.13 ppmv.
The arrurancy of FISH is 6% * value + 0,2 ppmv.

More details of the instrument and the calibration procedure are described in Zöger et al. [1999]
 

 


Updated 15-Oct-2008.

 
                                                                                  

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